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Publication Details
AFRICAN RESEARCH NEXUS
SHINING A SPOTLIGHT ON AFRICAN RESEARCH
earth and planetary sciences
Quantifying the contribution of marine organic gases to atmospheric iodine
Geophysical Research Letters, Volume 37, No. 18, Article L18804, Year 2010
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Description
Oceanic emissions of gaseous organic iodine-atom precursors have the potential to significantly affect atmospheric chemistry and climate, however there is currently considerable uncertainty associated with quantifying their sources. We present sea-air fluxes calculated from simultaneous air and seawater measurements of a comprehensive range of volatile organic iodine compounds (VOICs), including CH3I and the less commonly reported dihalomethanes CH2ICl, CH2IBr and CH2I2, made during two cruises in the Atlantic Ocean between 15-58N. The combined dihalomethane flux provides a global iodine source (∼0.33 0.19 Tg I y -1) comparable to that of CH3I, and a surface iodine atom source 3-4 times higher. However, a 1D atmospheric model reveals that, in the tropical east Atlantic Ocean in the vicinity of Cape Verde, even these combined VOIC fluxes are capable of supporting only ∼10-25% of the observed IO levels, and suggests that a substantial (340-640 nmol I m-2 d -1) additional photochemical source of iodine is required. © 2010 by the American Geophysical Union.
Authors & Co-Authors
Jones, Charlotte Emily
United Kingdom, York
University of York
Sommariva, Roberto
United Kingdom, Norwich
University of East Anglia
Dunk, Rachel M.
United Kingdom, York
University of York
von Glasow, Roland
United Kingdom, Norwich
University of East Anglia
McFiggans, G. B.
United Kingdom, Manchester
The University of Manchester
Carpenter, Lucy J.
United Kingdom, York
University of York
Statistics
Citations: 94
Authors: 6
Affiliations: 4
Identifiers
Doi:
10.1029/2010GL043990
ISSN:
00948276
Research Areas
Environmental
Study Locations
Cabo Verde