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Publication Details
AFRICAN RESEARCH NEXUS
SHINING A SPOTLIGHT ON AFRICAN RESEARCH
chemistry
LT-LiNi1/3Mn1/3Co1/3O2: A Partially-Disordered, Composite Rock Salt Cathode Prepared by Flame Spray Pyrolysis for Li-Ion Batteries
Journal of the Electrochemical Society, Volume 170, No. 5, Article 050511, Year 2023
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Description
A unique composite cathode structure for Li-ion batteries, designated LT-LiNi1/3Mn1/3Co1/3O2 (or LT-NMC111), has been prepared by flame spray pyrolysis and subsequent annealing between 400 and 650 °C. It is composed predominantly of structurally-integrated and partially-disordered lithiated-spinel and layered components, both of which can be broadly described as partially-disordered rock salt constituents. The paper describes the evolution of the LT-NMC111 structure as a function of the synthesis method, annealing temperature, and electrochemical properties in the context of other recently reported “low-temperature” (LT) materials, such as LT-LiCo1−xAlxO2 and LT-LiMn0.5Ni0.5O2 or, in spinel notation, LT-Li2Co2-2xAl2xO4 and LT-Li2MnNiO4, respectively. © 2023 The Author(s). Published on behalf of The Electrochemical Society by IOP Publishing Limited.
Authors & Co-Authors
Li, Linze
United States, Richland
Environmental Molecular Sciences Laboratory
Gim, Jihyeon
United States, Lemont
Argonne National Laboratory
Croy, Jason R.
United States, Lemont
Argonne National Laboratory
Thackeray, Michaelm M.
United States, Lemont
Argonne National Laboratory
Statistics
Authors: 4
Affiliations: 3
Identifiers
Doi:
10.1149/1945-7111/acd02e
ISSN:
00134651